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Assessment of Efficiency of Rare Earth Elements Recovery from Lignite Coal Combustion Ash via Five-Stage Extraction

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2021
397.pdf (948.9Kb)
Authors
Miličić, Ljiljana
Terzić, Anja
Pezo, Lato
Mijatović, Nevenka
Brceski, Ilija
Vukelić, Nikola
Article (Published version)
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Abstract
Rare earth elements (REE) are frequently referred to as ingredients for enhancements in modem industry, as they are extensively applied in many industrial branches due to their accented electro-magnetic and optical properties. REE have end-utilizations as catalysts, magnets, and as dopants for ceramic materials. Rare earth minerals are scarce therefore the unconventional REE-containing resources such as waste materials and industrial byproducts are continuously being investigated. Coal combustion products comprise REE concentrations varying between 200 ppm and 1500 ppm. This quantity can be isolated though the extraction procedure. In this study, the five stages extraction was conducted on the coal combustion ash from the selected landfill site. The extractions of 32 elements (As, Ga, Ce, Be, Ge, Nd, Cr, Zr, Eu, Cu, Nb, Gd, Co, Mo, Dy, Li, Ag, W, Mn, Cd, Au, Ni, In, Hg, Pb, Sn, Ti, V, Sb, Th, Zn, and La) were conveyed. Chemical analyses were conducted via XRF, ICP-OES, ICP-MS, and MS t...echniques. The complexity of the obtained data was examined by Principal component analysis and Cluster analysis in order to derive interconnections between quantity of elements and landfill characteristics, as well as mutual relationships among the elements of interest, and to assess the accomplishment of REE recovery from the coal ash.

Keywords:
Powdery materials / Industrial byproduct / Dopants for ceramic materials / Chemical extraction / Analytical modeling
Source:
Science of Sintering, 2021, 53, 2, 169-185
Publisher:
  • Međunarodni Institut za nauku o sinterovanju, Beograd
Funding / projects:
  • Ministry of Education, Science and Technological Development, Republic of Serbia, Grant no. 200012 (Istitute of Material Testing of Serbia - IMS, Belgrade) (RS-200012)

DOI: 10.2298/SOS2102169M

ISSN: 0350-820X

WoS: 000691836600003

Scopus: 2-s2.0-85110498766
[ Google Scholar ]
1
URI
http://rims.institutims.rs/handle/123456789/400
Collections
  • Radovi istraživača / Researchers' publications
Institution/Community
Institut za ispitivanje materijala
TY  - JOUR
AU  - Miličić, Ljiljana
AU  - Terzić, Anja
AU  - Pezo, Lato
AU  - Mijatović, Nevenka
AU  - Brceski, Ilija
AU  - Vukelić, Nikola
PY  - 2021
UR  - http://rims.institutims.rs/handle/123456789/400
AB  - Rare earth elements (REE) are frequently referred to as ingredients for enhancements in modem industry, as they are extensively applied in many industrial branches due to their accented electro-magnetic and optical properties. REE have end-utilizations as catalysts, magnets, and as dopants for ceramic materials. Rare earth minerals are scarce therefore the unconventional REE-containing resources such as waste materials and industrial byproducts are continuously being investigated. Coal combustion products comprise REE concentrations varying between 200 ppm and 1500 ppm. This quantity can be isolated though the extraction procedure. In this study, the five stages extraction was conducted on the coal combustion ash from the selected landfill site. The extractions of 32 elements (As, Ga, Ce, Be, Ge, Nd, Cr, Zr, Eu, Cu, Nb, Gd, Co, Mo, Dy, Li, Ag, W, Mn, Cd, Au, Ni, In, Hg, Pb, Sn, Ti, V, Sb, Th, Zn, and La) were conveyed. Chemical analyses were conducted via XRF, ICP-OES, ICP-MS, and MS techniques. The complexity of the obtained data was examined by Principal component analysis and Cluster analysis in order to derive interconnections between quantity of elements and landfill characteristics, as well as mutual relationships among the elements of interest, and to assess the accomplishment of REE recovery from the coal ash.
PB  - Međunarodni Institut za nauku o sinterovanju, Beograd
T2  - Science of Sintering
T1  - Assessment of Efficiency of Rare Earth Elements Recovery from Lignite Coal Combustion Ash via Five-Stage Extraction
EP  - 185
IS  - 2
SP  - 169
VL  - 53
DO  - 10.2298/SOS2102169M
UR  - conv_513
ER  - 
@article{
author = "Miličić, Ljiljana and Terzić, Anja and Pezo, Lato and Mijatović, Nevenka and Brceski, Ilija and Vukelić, Nikola",
year = "2021",
abstract = "Rare earth elements (REE) are frequently referred to as ingredients for enhancements in modem industry, as they are extensively applied in many industrial branches due to their accented electro-magnetic and optical properties. REE have end-utilizations as catalysts, magnets, and as dopants for ceramic materials. Rare earth minerals are scarce therefore the unconventional REE-containing resources such as waste materials and industrial byproducts are continuously being investigated. Coal combustion products comprise REE concentrations varying between 200 ppm and 1500 ppm. This quantity can be isolated though the extraction procedure. In this study, the five stages extraction was conducted on the coal combustion ash from the selected landfill site. The extractions of 32 elements (As, Ga, Ce, Be, Ge, Nd, Cr, Zr, Eu, Cu, Nb, Gd, Co, Mo, Dy, Li, Ag, W, Mn, Cd, Au, Ni, In, Hg, Pb, Sn, Ti, V, Sb, Th, Zn, and La) were conveyed. Chemical analyses were conducted via XRF, ICP-OES, ICP-MS, and MS techniques. The complexity of the obtained data was examined by Principal component analysis and Cluster analysis in order to derive interconnections between quantity of elements and landfill characteristics, as well as mutual relationships among the elements of interest, and to assess the accomplishment of REE recovery from the coal ash.",
publisher = "Međunarodni Institut za nauku o sinterovanju, Beograd",
journal = "Science of Sintering",
title = "Assessment of Efficiency of Rare Earth Elements Recovery from Lignite Coal Combustion Ash via Five-Stage Extraction",
pages = "185-169",
number = "2",
volume = "53",
doi = "10.2298/SOS2102169M",
url = "conv_513"
}
Miličić, L., Terzić, A., Pezo, L., Mijatović, N., Brceski, I.,& Vukelić, N.. (2021). Assessment of Efficiency of Rare Earth Elements Recovery from Lignite Coal Combustion Ash via Five-Stage Extraction. in Science of Sintering
Međunarodni Institut za nauku o sinterovanju, Beograd., 53(2), 169-185.
https://doi.org/10.2298/SOS2102169M
conv_513
Miličić L, Terzić A, Pezo L, Mijatović N, Brceski I, Vukelić N. Assessment of Efficiency of Rare Earth Elements Recovery from Lignite Coal Combustion Ash via Five-Stage Extraction. in Science of Sintering. 2021;53(2):169-185.
doi:10.2298/SOS2102169M
conv_513 .
Miličić, Ljiljana, Terzić, Anja, Pezo, Lato, Mijatović, Nevenka, Brceski, Ilija, Vukelić, Nikola, "Assessment of Efficiency of Rare Earth Elements Recovery from Lignite Coal Combustion Ash via Five-Stage Extraction" in Science of Sintering, 53, no. 2 (2021):169-185,
https://doi.org/10.2298/SOS2102169M .,
conv_513 .

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